Administration of EMP-related Publications
year | 2021 |
author(s) | R. Ohlendorf, S. Spachmann, L. Fischer, K. Dey, D. Brunt, G. Balakrishnan, O. A. Petrenko, R. Klingeler |
title | Magnetoelastic coupling and Grüneisen scaling in NdB4 |
document type | Paper |
source | Phys. Rev. B 103, 104424 (2021) |
doi | 10.1103/PhysRevB.103.104424 |
arxiv | https://arxiv.org/abs/2012.00723 |
EMP/Horizon2020 | This publication does not include a EMP/Horizon2020 acknowledgement. |
abstract | We report high-resolution capacitance dilatometry studies on the uniaxial length changes in a NdB4 single crystal. The evolution of magnetically ordered phases below TN= 17.2~K (commensurate antiferromagnetic phase, cAFM), TIT= 6.8~K (intermediate incommensurate phase, IT), and TLT= 4.8~K (low-temperature phase, LT) is associated with pronounced anomalies in the thermal expansion coefficients. The data imply significant magneto-elastic coupling and evidence of a structural phase transition at TLT . While both cAFM and LT favor structural anisotropy δ between in-plane and out-of-plane length changes, it competes with the IT-type of order, i.e., δ is suppressed in that phase. Notably, finite anisotropy well above TN indicates short-range correlations which are, however, of neither cAFM, IT, nor LT-type. Grüneisen analysis of the ratio of thermal expansion coefficient and specific heat enables the derivation of uniaxial as well as hydrostatic pressure dependencies. While α/cp evidences a single dominant energy scale in LT, our data imply precursory fluctuations of a competing phase in IT and cAFM, respectively. Our results suggest the presence of orbital degrees of freedom competing with cAFM and successive evolution of a magnetically and orbitally ordered ground state. |